Search for: All records

Magnons, the quanta of collective spin excitations in magnetic materials, may enable functionalities, such as nonreciprocity and transduction in hybrid quantum devices. To assess the potential of such applications, it is necessary to understand magnon dynamics beyond the simple harmonic oscillator regime, where theory predicts effects like population-dependent damping and quantum fluctuations in the form of magnon shot noise. Probing these phenomena requires sensors with high sensitivity and the ability to resolve magnon properties across different excitation regimes. Here, we demonstrate accurate and sensitive detection of magnon population and decay over a wide range of occupation numbers. We use a superconducting qubit to probe magnons in a ferrimagnet over approximately 2000 excitations. Using qubit control and parametrically induced qubit-magnon interactions, we demonstrate few-excitation sensitive detection of magnons with a dynamic range of approximately 30 dB, and are able to accurately resolve their decay with few-ns sensitivity. These capabilities offer a powerful and practical technique for probing magnon dynamics in or beyond the linear regime over a wide range of excitations. 

Nonreciprocal microwave routing plays a crucial role in measuring quantum circuits, and allows for realizing cascaded quantum systems for generating and stabilizing entanglement between noninteracting qubits. The most commonly used tools for implementing directionality are ferrite-based circulators. These devices are versatile, but suffer from excess loss, a large footprint, and fixed directionality. For utilizing nonreciprocity in scalable quantum circuits it is desirable to develop efficient integration of low-loss and controllable directional elements. Here, we report the design and experimental realization of a minimal controllable directional interface that can be directly coupled to superconducting qubits. In the device presented, nonreciprocity is realized through a combination of interference and phase-controlled parametric pumping. We have achieved a maximum directionality of around 30 dB, and the performance of the device is predicted quantitatively from independent calibration measurements. Using the excellent agreement of model and experiment, we predict that the circuit will be useable as a chiral qubit interface with inefficiencies at the $1\mathrm{\%}$level or below. Our work offers a promising route for realizing high-fidelity signal routing and entanglement generation in all-to-all connected microwave quantum networks, and provides a path for isolator-free qubit readout schemes. Published by the American Physical Society2024 

Establishing limits of entanglement in open quantum systems is a problem of fundamental interest, with strong implications for applications in quantum information science. Here, we study the limits of entanglement stabilization between remote qubits. We theoretically investigate the loss resilience of driven-dissipative entanglement between remote qubits coupled to a chiral waveguide. We find that by coupling a pair of storage qubits to the two driven qubits, the steady state can be tailored such that the storage qubits show a degree of entanglement that is higher than what can be achieved with only two driven qubits coupled to the waveguide. By reducing the degree of entanglement of the driven qubits, we show that the entanglement between the storage qubits becomes more resilient to waveguide loss. Our analytical and numerical results offer insights into how waveguide loss limits the degree of entanglement in this driven-dissipative system, and they offer important guidance for remote entanglement stabilization in the laboratory, for example using superconducting circuits. Published by the American Physical Society2024 

Abstract One of the primary challenges in realizing large-scale quantum processors is the realization of qubit couplings that balance interaction strength, connectivity, and mode confinement. Moreover, it is very desirable for the device elements to be detachable, allowing components to be built, tested, and replaced independently. In this work, we present a microwave quantum state router, centered on parametrically driven, Josephson-junction based three-wave mixing, that realizes all-to-all couplings among four detachable quantum modules. We demonstrate coherent exchange among all four communication modes, with an average full-iSWAP time of 764 ns and average inferred inter-module exchange fidelity of 0.969, limited by mode coherence. We also demonstrate photon transfer and pairwise entanglement between module qubits, and parallel operation of simultaneousiSWAP exchange across the router. Our router-module architecture serves as a prototype of modular quantum computer that has great potential for enabling flexible, demountable, large-scale quantum networks of superconducting qubits and cavities. 

Abstract Atmospheric rivers (ARs) reaching high-latitudes in summer contribute to the majority of climatological poleward water vapor transport into the Arctic. This transport has exhibited long term changes over the past decades, which cannot be entirely explained by anthropogenic forcing according to ensemble model responses. Here, through observational analyses and model experiments in which winds are adjusted to match observations, we demonstrate that low-frequency, large-scale circulation changes in the Arctic play a decisive role in regulating AR activity and thus inducing the recent upsurge of this activity in the region. It is estimated that the trend in summertime AR activity may contribute to 36% of the increasing trend of atmospheric summer moisture over the entire Arctic since 1979 and account for over half of the humidity trends in certain areas experiencing significant recent warming, such as western Greenland, northern Europe, and eastern Siberia. This indicates that AR activity, mostly driven by strong synoptic weather systems often regarded as stochastic, may serve as a vital mechanism in regulating long term moisture variability in the Arctic. 

Abstract Due to their high coherence, lasers are ubiquitous tools in science. We show that by engineering the coupling between the gain medium and the laser cavity as well as the laser cavity and the output port, it is possible to eliminate most of the noise due to photons entering as well as leaving the laser cavity. Hence, it is possible to reduce the laser linewidth by a factor equal to the number of photons in the laser cavity below the standard quantum limit. We design and theoretically analyze a superconducting circuit that uses Josephson junctions, capacitors and inductors to implement a microwave laser, including the low-noise couplers that allow the design to surpass the standard quantum limit. Our proposal relies on the elements of superconducting quantum information, and thus is an example of how quantum engineering techniques can inspire us to re-imagine the limits of conventional quantum systems. 

Water splitting has been widely considered to be an efficient way to generate sustainable and renewable energy resources in fuel cells, metal–air batteries and other energy conversion devices. Exploring efficient electrocatalysts to expedite the anodic oxygen evolution reaction (OER) is a crucial task that needs to be addressed in order to boost the practical application of water splitting. Intensive efforts have been devoted to develop mixed transition metal based chalcogenides as effective OER electrocatalysts. Herein, we have reported synthesis of a series of mixed metal selenides containing Co, Ni and Cu employing combinatorial electrodeposition, and systematically investigated how the transition metal doping affects the OER catalytic activity in alkaline medium. Energy dispersive spectroscopy (EDS) was performed to detect the elemental compositions and confirm the feasibility of compositional control of 66 metal selenide thin films. It was observed that the OER catalytic activity is sensitive to the concentration of Cu in the catalysts, and the catalyst activity tended to increase with increasing Cu concentration. However, increasing the Cu concentration beyond a certain limit led to decrease in catalytic efficiency, and copper selenide by itself, although catalytically active, showed higher onset potential and overpotential for OER compared to the ternary and quaternary mixed metal selenides. Interestingly, the best quaternary composition (Co 0.21 Ni 0.25 Cu 0.54 ) 3 Se 2 showed similar crystal structure as its parent compound of Cu 3 Se 2 with slight decrease in lattice spacings of (101) and (210) lattice planes (0.0222 Å and 0.0148 Å, respectively) evident from the powder X-ray diffraction pattern. (Co 0.21 Ni 0.25 Cu 0.54 ) 3 Se 2 thin film exhibited excellent OER catalytic activity and required an overpotential of 272 mV to reach a current density of 10 mA cm −2 , which is 54 mV lower than Cu 3 Se 2 , indicating a synergistic effect of transition metal doping in enhancing catalytic activity.